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1.
Atmospheric Chemistry and Physics ; 23(8):4863-4880, 2023.
Article in English | ProQuest Central | ID: covidwho-2298817

ABSTRACT

The global atmospheric methane growth rates reported by NOAA for 2020 and 2021 are the largest since systematic measurements began in 1983. To explore the underlying reasons for these anomalous growth rates, we use newly available methane data from the Japanese Greenhouse gases Observing SATellite (GOSAT) to estimate methane surface emissions. Relative to baseline values in 2019, we find that a significant global increase in methane emissions of 27.0 ± 11.3 and 20.8 ± 11.4 Tg is needed to reproduce observed atmospheric methane in 2020 and 2021, respectively, assuming fixed climatological values for OH. We see the largest annual increases in methane emissions during 2020 over Eastern Africa (14 ± 3 Tg), tropical Asia (3 ± 4 Tg), tropical South America (5 ± 4 Tg), and temperate Eurasia (3 ± 3 Tg), and the largest reductions are observed over China (-6 ± 3 Tg) and India (-2 ± 3 Tg). We find comparable emission changes in 2021, relative to 2019, except for tropical and temperate South America where emissions increased by 9 ± 4 and 4 ± 3 Tg, respectively, and for temperate North America where emissions increased by 5 ± 2 Tg. The elevated contributions we saw in 2020 over the western half of Africa (-5 ± 3 Tg) are substantially reduced in 2021, compared to our 2019 baseline. We find statistically significant positive correlations between anomalies of tropical methane emissions and groundwater, consistent with recent studies that have highlighted a growing role for microbial sources over the tropics. Emission reductions over India and China are expected in 2020 due to the Covid-19 lockdown but continued in 2021, which we do not currently understand. To investigate the role of reduced OH concentrations during the Covid-19 lockdown in 2020 on the elevated atmospheric methane growth in 2020–2021, we extended our inversion state vector to include monthly scaling factors for OH concentrations over six latitude bands. During 2020, we find that tropospheric OH is reduced by 1.4 ± 1.7 % relative to the corresponding 2019 baseline value. The corresponding revised global growth of a posteriori methane emissions in 2020 decreased by 34 % to 17.9 ± 13.2 Tg, relative to the a posteriori value that we inferred using fixed climatological OH values, consistent with sensitivity tests using the OH climatology inversion using reduced values for OH. The counter statement is that 66 % of the global increase in atmospheric methane during 2020 was due to increased emissions, particularly from tropical regions. Regional flux differences between the joint methane–OH inversion and the OH climatology inversion in 2020 are typically much smaller than 10 %. We find that OH is reduced by a much smaller amount during 2021 than in 2020, representing about 10 % of the growth of atmospheric methane in that year. Therefore, we conclude that most of the observed increase in atmospheric methane during 2020 and 2021 is due to increased emissions, with a significant contribution from reduced levels of OH.

2.
Atmospheric Chemistry and Physics ; 20(24):15743-15759, 2020.
Article in English | ProQuest Central | ID: covidwho-1022162

ABSTRACT

We report changes in surface nitrogen dioxide (NO2) across the UK during the COVID-19 pandemic when large and rapid emission reductions accompanied a nationwide lockdown (23 March–31 May 2020, inclusively), and compare them with values from an equivalent period over the previous 5 years. Data are from the Automatic Urban and Rural Network (AURN), which forms the basis of checking nationwide compliance with ambient air quality directives. We calculate thatNO2 reduced by 42%±9.8% on average across all 126 urban AURN sites, with a slightly larger (48%±9.5%) reduction at sites close to the roadside (urban traffic). We also find that ozone (O3) increased by 11 % on average across the urban background network during the lockdown period. Total oxidant levels (Ox=NO2+O3) increased only slightly on average (3.2%±0.2%), suggesting the majority of this change can be attributed to photochemical repartitioning due to the reduction in NOx. Generally, we find larger, positiveOx changes in southern UK cities, which we attribute to increased UV radiation and temperature in 2020 compared to previous years. The net effect of the NO2 andO3 changes is a sharp decrease in exceedances of the NO2 air quality objective limit for the UK, with only one exceedance in London in 2020 up until the end of May. Concurrent increases in O3 exceedances in London emphasize the potential for O3 to become an air pollutant of concern as NOx emissions are reduced in the next 10–20 years.

3.
Friedlingstein, Pierre, O'Sullivan, Michael, Jones, Matthew W.; Andrew, Robbie M.; Hauck, Judith, Olsen, Are, Peters, Glen P.; Peters, Wouter, Pongratz, Julia, Sitch, Stephen, Corinne, Le Quéré, Canadell, Josep G.; Ciais, Philippe, Jackson, Robert B.; Alin, Simone, Luiz E O , C. Aragão, Arneth, Almut, Arora, Vivek, Bates, Nicholas R.; Becker, Meike, Benoit-Cattin, Alice, Bittig, Henry C.; Bopp, Laurent, Bultan, Selma, Chandra, Naveen, Chevallier, Frédéric, Chini, Louise P.; Evans, Wiley, Florentie, Liesbeth, Forster, Piers M.; Gasser, Thomas, Gehlen, Marion, Gilfillan, Dennis, Gkritzalis, Thanos, Luke, Gregor, Gruber, Nicolas, Harris, Ian, Hartung, Kerstin, Haverd, Vanessa, Houghton, Richard A.; Ilyina, Tatiana, Jain, Atul K.; Joetzjer, Emilie, Kadono, Koji, Kato, Etsushi, Kitidis, Vassilis, Korsbakken, Jan Ivar, Landschützer, Peter, Lefèvre, Nathalie, Lenton, Andrew, Lienert, Sebastian, Liu, Zhu, Lombardozzi, Danica, Marland, Gregg, Metzl, Nicolas, Munro, David R.; Julia E M , S. Nabel, Shin-Ichiro, Nakaoka, Niwa, Yosuke, O'Brien, Kevin, Ono, Tsuneo, Palmer, Paul I.; Pierrot, Denis, Poulter, Benjamin, Resplandy, Laure, Robertson, Eddy, Rödenbeck, Christian, Schwinger, Jörg, Séférian, Roland, Skjelvan, Ingunn, Smith, Adam J. P.; Sutton, Adrienne J.; Toste, Tanhua, Tans, Pieter P.; Tian, Hanqin, Tilbrook, Bronte, van der Werf, Guido, Vuichard, Nicolas, Walker, Anthony P.; Wanninkhof, Rik, Watson, Andrew J.; Willis, David, Wiltshire, Andrew J.; Yuan, Wenping, Xu, Yue, Zaehle, Sönke.
Earth System Science Data ; 12(4):3269-3340, 2020.
Article in English | ProQuest Central | ID: covidwho-971932

ABSTRACT

Accurate assessment of anthropogenic carbon dioxide (CO2) emissions and their redistribution among the atmosphere, ocean, and terrestrial biosphere in a changing climate – the “global carbon budget” – is important to better understand the global carbon cycle, support the development of climate policies, and project future climate change. Here we describe and synthesize data sets and methodology to quantify the five major components of the global carbon budget and their uncertainties. Fossil CO2 emissions (EFOS) are based on energy statistics and cement production data, while emissions from land-use change (ELUC), mainly deforestation, are based on land use and land-use change data and bookkeeping models. Atmospheric CO2 concentration is measured directly and its growth rate (GATM) is computed from the annual changes in concentration. The ocean CO2 sink (SOCEAN) and terrestrial CO2 sink (SLAND) are estimated with global process models constrained by observations. The resulting carbon budget imbalance (BIM), the difference between the estimated total emissions and the estimated changes in the atmosphere, ocean, and terrestrial biosphere, is a measure of imperfect data and understanding of the contemporary carbon cycle. All uncertainties are reported as ±1σ. For the last decade available (2010–2019), EFOS was 9.6 ± 0.5 GtC yr-1 excluding the cement carbonation sink (9.4 ± 0.5 GtC yr-1 when the cement carbonation sink is included), andELUC was 1.6 ± 0.7 GtC yr-1. For the same decade, GATM was 5.1 ± 0.02 GtC yr-1 (2.4 ± 0.01 ppm yr-1), SOCEAN 2.5 ± 0.6 GtC yr-1, and SLAND 3.4 ± 0.9 GtC yr-1, with a budget imbalance BIM of -0.1 GtC yr-1 indicating a near balance between estimated sources and sinks over the last decade. For the year 2019 alone, the growth in EFOS was only about 0.1 % with fossil emissions increasing to 9.9 ± 0.5 GtC yr-1 excluding the cement carbonation sink (9.7 ± 0.5 GtC yr-1 when cement carbonation sink is included), and ELUC was 1.8 ± 0.7 GtC yr-1, for total anthropogenic CO2 emissions of 11.5 ± 0.9 GtC yr-1 (42.2 ± 3.3 GtCO2). Also for 2019, GATM was 5.4 ± 0.2 GtC yr-1 (2.5 ± 0.1 ppm yr-1), SOCEAN was 2.6 ± 0.6 GtC yr-1, and SLAND was 3.1 ± 1.2 GtC yr-1, with a BIM of 0.3 GtC. The global atmospheric CO2 concentration reached 409.85 ± 0.1 ppm averaged over 2019. Preliminary data for 2020, accounting for the COVID-19-induced changes in emissions, suggest a decrease in EFOS relative to 2019 of about -7 % (median estimate) based on individual estimates from four studies of -6 %, -7 %,-7 % (-3 % to -11 %), and -13 %. Overall, the mean and trend in the components of the global carbon budget are consistently estimated over the period 1959–2019, but discrepancies of up to 1 GtC yr-1 persist for the representation of semi-decadal variability in CO2 fluxes. Comparison of estimates from diverse approaches and observations shows (1) no consensus in the mean and trend in land-use change emissions over the last decade, (2) a persistent low agreement between the different methods on the magnitude of the land CO2 flux in the northern extra-tropics, and (3) an apparent discrepancy between the different methods for the ocean sink outside the tropics, particularly in the Southern Ocean. This living data update documents changes in the methods and data sets used in this new global carbon budget and the progress in understanding of the global carbon cycle compared with previous publications of this data set (Friedlingstein et al., 2019;Le Quéré et al., 2018b, a, 2016, 2015b, a, 2014, 2013). The data presented in this work are available at 10.18160/gcp-2020 (Friedlingstein et al., 2020).

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